• 摘要: 过渡金属硫族化物(Transition metal dichalcogenides, TMDCs)作为典型二维范德瓦尔斯材料,因独特能带结构与良好的光学性质而受到广泛关注。与单层体系相比,块体/多层 TMDCs 兼具高折射率与激子,在可见—近红外波段表现出强光–物质相互作用的显著优势。近年来,围绕 TMDCs 的强耦合研究迅速推进,已在米氏共振,法布里-珀罗腔,准束缚态等光学模式中实现与激子的强耦合。本文聚焦块体/多层 TMDCs 强耦合领域,系统梳理其最新研究进展,总结了不同光学腔体系(表面等离激元腔、法布里–珀罗腔及高折射率介质谐振腔/纳米天线)的研究,并对未来发展趋势进行了展望。

       

      Abstract: Transition-metal dichalcogenides (TMDCs), as prototypical two-dimensional van der Waals materials, have attracted widespread attention because of their distinctive electronic band structures and excellent optical properties. Compared with monolayers, bulk and multilayer TMDCs combine a high refractive index with robust excitonic responses, thereby enabling pronounced light-matter interactions over the visible-to-near-infrared range. In recent years, studies of strong coupling in TMDCs have progressed rapidly, achieving strong coupling between excitons and optical modes such as Mie resonances, Fabry–Pérot (FP) cavities, and quasi-bound states in the continuum. This article focuses on strong coupling in bulk/multilayer TMDCs, provides a systematic overview of the latest advances, summarizes research across different optical cavity platforms—including plasmonic cavities, FP cavities, and high-index dielectric resonators/nanoantennas—and offers an outlook on future developments.