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Optical bubble, characterized by a tightly focused three-dimensional dark-field spot distribution, exhibits significant application values in fields such as optical manipulation and laser processing. Since 2000, research on the focused field distribution of optical bubbles has gradually gained attention. Arlt et al. generated an optical bubble in the focal region through the coherent superposition of two different Laguerre-Gaussian beam modes. Zhan et al. produced a tightly focused optical bubble using cylindrical vector beams combined with binary diffractive optical elements. Kozawa et al. achieved an optical bubble via coherent superposition of double annular radially polarized beams. However, the poor intensity uniformity at the edges of these generated bubbles limits their practical applicability. Bokor et al. utilized a Laguerre-Gaussian radially polarized beam for 4π focusing, generating an optical bubble with high intensity uniformity in the focal region. However, the counter-propagating focusing scheme in 4π focusing requires extremely high experimental alignment precision, making it challenging to implement in practice. Subsequently, this research group achieved the generation of an optical bubble with high intensity uniformity under conventional unidirectional focusing conditions by adjusting the energy ratio between an azimuthally polarized incident beam and a radially polarized incident beam modulated by a 0/π binary phase. Nevertheless, current experimental realizations of optical bubbles rely on multi-beam synthesis, which imposes stringent requirements on the experimental setup, particularly the multi-pulse beam synthesis system.
To address this issue, we utilize single-beam vector field modulation technology to generate an optical bubble with high intensity uniformity in a simplified experimental system. Furthermore, polarization conversion of the probe light enables the detection of individual polarization components within the focused field, facilitating the reconstruction of the three-dimensional morphology distribution of the optical bubble. By optimizing the energy ratio between the azimuthally polarized incident beam and the radially polarized incident beam modulated by a 0/π binary phase, we experimentally demonstrate an optical bubble with an edge-to-center dark spot intensity ratio exceeding 10:1 and edge intensity uniformity approaching 90%. Highly uniform optical bubble significantly enhances particle manipulation by enabling precise trapping of particles, thereby improving experimental controllability and repeatability. In terms of processing accuracy, it mitigates issues such as non-uniform machining depth and edge burrs, ultimately increasing production yield in material processing applications. Compared to traditional multi-beam synthesis methods, this technology markedly reduces system complexity while doubling optical energy utilization efficiency, providing a more practical technical approach for applications in dual-beam super-resolution laser processing, optical data storage, and particle manipulation.
Normalized intensity distributions of optical field intensity in XY focal plane and XZ plane containing the optical axis, as well as theoretical results of normalized intensity curves of three-dimensional optical bubble. (a) Tightly focused hollow tubular optical field generated by azimuthally polarized incident beam; (b) Tightly focused optical field generated by radially polarized incident beam with 0/π binary phase modulation; (c) Tightly focused three-dimensional optical bubble generated by superposition of two under optimal intensity uniformity;(d) Variation curve of three-dimensional optical bubble uniformity under different energy ratios (RP/AP); (e) Normalized intensity curves of three-dimensional optical bubble along x-direction, z-direction, and c-direction
Optical path schematic for the generation and detection of a tightly focused optical bubble based on single-path vector beams manipulation and gold nanoparticle scanning
Experimental results of normalized intensity distributions of optical field in XY focal plane and XZ plane containing optical axis, as well as normalized intensity curves of three-dimensional optical bubble. (a) Tightly focused hollow tubular optical field generated by azimuthally polarized incident beam; (b) Tightly focused optical field generated by radially polarized incident beam with 0/π binary phase modulation;(c) Tightly focused optical bubble generated by the superposition of the two; Normalized intensity curves of three-dimensional optical bubble along (d) x-direction, (e) z-direction, and (f) c-direction